Nuclear waste from small modular reactors

Författare
Lindsay M. Krall
Allison M. Macfarlane
Rodney C. Ewing
2022-05-31

PDF (12 pp., 1.62 MB)

Source: https://www.pnas.org/doi/full/10.1073/pnas.2111833119

Nuclear waste from small modular reactors

Lindsay M. Krall , Allison M. Macfarlane, and Rodney C. Ewinga
Edited by Eric J. Schelter, University of Pennsylvania, Philadelphia, PA; received June 26, 2021; accepted March 17, 2022 by Editorial Board Member
Peter J. Rossky

Significance

Small modular reactors (SMRs), proposed as the future of nuclear energy, have purported cost and safety advantages over existing gigawatt-scale light water reactors (LWRs). However, few studies have assessed the implications of SMRs for the back end of the nuclear fuel cycle. The low-, intermediate-, and high-level waste stream characterization presented here reveals that SMRs will produce more voluminous and chemically/physically reactive waste than LWRs, which will impact options for the management and disposal of this waste. Although the analysis focuses on only three of dozens of proposed SMR designs, the intrinsically higher neutron leakage associated with SMRs suggests that most designs are inferior to LWRs with respect to the generation, management, and final disposal of key radionuclides in nuclear waste.

Abstract

Small modular reactors (SMRs; i.e., nuclear reactors that produce <300 MWelec each) have garnered attention because of claims of inherent safety features and reduced cost. However, remarkably few studies have analyzed the management and disposal of their nuclear waste streams. Here, we compare three distinct SMR designs to an 1,100-MWelec pressurized water reactor in terms of the energy-equivalent volume, (radio-)chemistry, decay heat, and fissile isotope composition of (notional) high-, intermediate-, and low-level waste streams. Results reveal that water-, molten salt–, and sodium-cooled SMR designs will increase the volume of nuclear waste in need of management and disposal by factors of 2 to 30. The excess waste volume is attributed to the use of neutron reflectors and/or of chemically reactive fuels and coolants in SMR designs. That said, volume is not the most important evaluation metric; rather, geologic repository performance is driven by the decay heat power and the (radio-)chemistry of spent nuclear fuel, for which SMRs provide no benefit. SMRs will not reduce the generation of geochemically mobile 129I, 99Tc, and 79Se fission products, which are important dose contributors for most repository designs. In addition, SMR spent fuel will contain relatively high concentrations of fissile nuclides, which will demand novel approaches to evaluating criticality during storage and disposal. Since waste stream properties are influenced by neutron leakage, a basic physical process that is enhanced in small reactor cores, SMRs will exacerbate the challenges of nuclear waste management and disposal.

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Response from proponents of SMRs:

Utgivningsår
2022
Bilaga Storlek
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